KubarychGroup
KubarychGroup
C.R. Baiz, M.J. Nee, R. McCanne, K.J. Kubarych, Opt. Lett. 33 (2008) 2533
We present what we believe to be the first implementation of nonequilibrium two-dimensional IR spectroscopy (2DIR) combining electronic excitation within the Fourier transform (FT) approach. Nonequilibrium 2DIR spectra of Mn2(CO)10 and its photoproducts are obtained in two modalities: photoexcitation at 400 nm, either before a 2DIR probe or during the waiting time of the FT 2DIR measurement. Extending FT 2DIR to nonequilibrium systems offers insight into complex condensed-phase reaction dynamics.
Ultrafast non-equilibrium Fourier-transform two-dimensional infrared spectroscopy
11/1/08